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- W4210610739 abstract "Abstract The development of controllable artificial light‐harvesting systems based on liquid crystal (LC) materials, i.e., anisotropic fluids, remains a challenge. Herein, an annulene‐based discotic LC compound 6 with a saddle‐shaped cyclooctatetrathiophene core has been synthesized to construct a tunable light‐harvesting platform. The LC material shows a typical aggregation‐induced emission, which can act as a suitable light‐harvesting donor. By loading Nile red (NiR) as an acceptor, an artificial light‐harvesting system is achieved. Relying on the thermal‐responsive self‐assembling ability of 6 with variable molecular order, the efficiency of such 6 ‐NiR system can be controlled by temperature. This light‐harvesting system works sensitively at a high donor/acceptor ratio as 1000 : 1, and exhibits a high antenna effect (39.1) at a 100 : 1 donor/acceptor ratio. This thermochromic artificial light‐harvesting LC system could find potential applications in smart devices employing soft materials." @default.
- W4210610739 created "2022-02-08" @default.
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- W4210610739 date "2022-02-15" @default.
- W4210610739 modified "2023-10-16" @default.
- W4210610739 title "An Artificial Light‐Harvesting System with Controllable Efficiency Enabled by an Annulene‐Based Anisotropic Fluid" @default.
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- W4210610739 doi "https://doi.org/10.1002/ange.202200466" @default.
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