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- W4210620797 abstract "Ion-exchange reactions are commonly used to develop novel metastable electrode materials for alkali-ion batteries that cannot be synthesized using direct chemical reactions. In this study, the electrochemical K to Na ion-exchange reaction mechanisms in a layered KxCoO2 cathode as a model system were investigated using operando and ex situ structure characterization techniques. Some level of K ions was observed to remain in the layered structure during the electrochemical ion-exchange reactions. Interestingly, the K ions are well separated from the Na-rich phases in the discharged state, and they form an intermediate phase in which K and Na ions are mixed at the top of charge. We discovered that such residual K ions prevent the collapse of the layered structure in the high-voltage regime, thereby improving the cycling stability in a Na-battery system." @default.
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- W4210620797 date "2022-05-01" @default.
- W4210620797 modified "2023-10-14" @default.
- W4210620797 title "Understanding of electrochemical K+/Na+ exchange mechanisms in layered oxides" @default.
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- W4210620797 doi "https://doi.org/10.1016/j.ensm.2022.01.057" @default.
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