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- W4210657455 abstract "Novel heterogeneous catalysts are needed to selectively anchor metal nanoparticles (NPs) into the internal space of carbon nanotubes (CNTs). Here, supercritical CO2 (SC-CO2) was used to fabricate the Ru@CNT composite microsponge via impregnation. Under SC-CO2 conditions, the highly dispersive Ru NPs, with a uniform diameter of 3 nm, were anchored exclusively into the internal space of CNTs. The CNTs are assembled into a microsponge composite. The supercritical temperature for catalyst preparation, catalytic hydrogenation temperature, and time all have a significant impact on the catalytic activity of Ru@CNTs. The best catalytic activity was obtained at 100 °C and 8.0 MPa: this gave excellent selectivity in the hydrogenation of p-chloronitrobenzene at 100 °C. This assembly strategy assisted by SC-CO2 will be promising for the fabrication of advanced carbon composite powder materials." @default.
- W4210657455 created "2022-02-08" @default.
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- W4210657455 date "2022-02-04" @default.
- W4210657455 modified "2023-10-14" @default.
- W4210657455 title "Ru@Carbon Nanotube Composite Microsponge: Fabrication in Supercritical CO2 for Hydrogenation of p-Chloronitrobenzene" @default.
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- W4210657455 doi "https://doi.org/10.3390/nano12030539" @default.
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