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- W4210709898 abstract "Abstract Transitional metals are widely used as co‐catalysts boosting photocatalytic H 2 production. However, metal‐based co‐catalysts suffer from high cost, limited abundance and detrimental environment impact. To date, metal‐free co‐catalyst is rarely reported. Here we for the first time utilized density functional calculations to guide the application of phosphorene as a high‐efficiency metal‐free co‐catalyst for CdS, Zn 0.8 Cd 0.2 S or ZnS. Particularly, phosphorene modified CdS shows a high apparent quantum yield of 34.7 % at 420 nm. This outstanding activity arises from the strong electronic coupling between phosphorene and CdS, as well as the favorable band structure, high charge mobility and massive active sites of phosphorene, supported by computations and advanced characterizations, for example, synchrotron‐based X‐ray absorption near edge spectroscopy. This work brings new opportunities to prepare highly‐active, cheap and green photocatalysts." @default.
- W4210709898 created "2022-02-08" @default.
- W4210709898 creator A5032509793 @default.
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- W4210709898 date "2017-07-19" @default.
- W4210709898 modified "2023-09-25" @default.
- W4210709898 title "Phosphorene Co‐catalyst Advancing Highly Efficient Visible‐Light Photocatalytic Hydrogen Production" @default.
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- W4210709898 doi "https://doi.org/10.1002/ange.201703827" @default.
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