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- W4210762405 abstract "Developing highly efficient bifunctional catalysts for the oxygen reduction and oxygen evolution reaction (ORR/OER) can open possibilities for future zinc air batteries (ZABs). Herein, cost-effective and highly conductive few-layer ferric and nickel chloride co-intercalated graphite intercalation compounds (FeCl3 -NiCl2 -GIC) are designed as bifunctional oxygen catalysts for ZAB. The optimized few-layer FeCl3 -NiCl2 -GIC catalyst exhibits a small overpotential of 276 mV at 10 mA cm-2 for the OER and achieves a high onset potential of 0.89 V for the ORR. The theoretical analysis demonstrates the electron-rich state on the carbon layers of FeCl3 -NiCl2 -GIC during the catalytic process favors the kinetics of electron transfer and lowers the absorption energy barriers for intermediates. Impressively, the ZAB assembled with few-layer FeCl3 -NiCl2 -GIC catalyst displays a 160 h cycling stability and a high energy efficiency of 72.6%. This work also suggests the possibility of utilizing layer electronic structure regulation on graphite intercalation compounds as effective bifunctional catalysts for ZABs." @default.
- W4210762405 created "2022-02-08" @default.
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- W4210762405 date "2022-01-31" @default.
- W4210762405 modified "2023-10-15" @default.
- W4210762405 title "Manipulating the Electronic Structure of Graphite Intercalation Compounds for Boosting the Bifunctional Oxygen Catalytic Performance" @default.
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- W4210762405 doi "https://doi.org/10.1002/smll.202107667" @default.
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