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- W4210794919 abstract "Plasmonic nanostructures with strong light absorption and high catalytic activity are ideal platform to realize efficient light-driven catalysis. This work developed a laser-induced-reshaping route (pulse width 10 ns, wavelength 1064 nm) to improve the efficiency of energy transfer between non-plasmonic material (Pt) and plasmonic Au nanorods (NRs). The catalytic performance for 4-nitrophenol (4-NP) hydrogenation was increased by 2-fold using laser-modified Pt-Au NRs (L-Pt-Au NRs) compared to original Pt-Au NRs. Very impressively, the relationship between laser-induced reshaping and resulting optical properties was investigated at single-particle level. Finite difference time domain (FDTD) simulation and single-particle photoluminescence (PL) quenching (48.6%) after laser induced reshaping, indicated the redistributed Pt atoms on Au NRs surfaces largely promoted hot electron transfer and decreased radiative photon re-emission. Further, the mechanism of plasmon-enhanced nitroreduction was studied in situ at the single-particle level. This work provides insight into the design and application of plasmonic nanostructures at single-particle level." @default.
- W4210794919 created "2022-02-08" @default.
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- W4210794919 date "2022-03-01" @default.
- W4210794919 modified "2023-10-16" @default.
- W4210794919 title "Boosting hot electrons transfer via laser-induced atomic redistribution for plasmon-enhanced nitroreduction and single-particle study" @default.
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- W4210794919 doi "https://doi.org/10.1016/j.jcat.2022.01.025" @default.
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