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• W4210873442 abstract "The oscillation continuum in laser-induced fluorescence spectra of bound-free c3Σ+ → a3Σ+ and (4)1Σ+ → X1Σ+ transitions of the KCs molecule was recorded by a Fourier-transform spectrometer and modeled under the adiabatic approximation. The required interatomic potentials for ground a3Σ+ and X1Σ+ states were reconstructed in an analytical Chebyshev-polynomial-expansion form in the framework of the regularization direct-potential-fit procedure based on the simultaneous consideration of experimental line positions from Ferber et al. [Phys. Rev. A 80, 062501 (2009)] and the present ab initio calculation of short-range repulsive potential data. It was proved that the repulsive part over the dissociation limit of the derived a3Σ+ potential reproduces the experiment better than the potentials reported in the literature. It is also shown that all empirical and semi-empirical potentials available for the X1Σ+ state reproduce the bound-free (4)1Σ+ → X1Σ+ spectrum with equal quality in the range of observations." @default.
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• W4210873442 date "2022-03-21" @default.
• W4210873442 modified "2023-09-23" @default.
• W4210873442 title "Observation and modeling of bound-free transitions to the <i>X</i>¹Σ⁺ and <i>a</i>³Σ⁺ states of KCs" @default.
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• W4210873442 doi "https://doi.org/10.1063/5.0082309" @default.
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