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- W4210919065 abstract "• Ion-irradiated ThO 2 is not uniform with respect to Raman spectroscopy, thus many points are analyzed to assess the damage. • Raman profiling of the damage depth agrees quite well with simulation predictions. Nuclear reactor conditions can be emulated in part by exposing potential fuel materials, such as ThO 2 , to ion beam radiation. Changes in properties can then provide invaluable insight into how the material will perform as a fuel. Here, a hydrothermally grown single crystal of ThO 2 is irradiated with 2 MeV H + and the crystallographic and electronic structure homogeneity and damage extent is investigated. μ-Raman spectroscopy shows that the damage to the crystal face directly exposed to the irradiation is heterogeneous, with the intensity of irradiation-induced peaks altering substantially in relation to the T 2g structural peak. Damage on orthogonal faces is more uniform and the damage depth profile is investigated with Raman spectroscopy. The damage as a function of depth is compared to stopping range of ions in matter simulations. Photoluminescence spectroscopy is also employed to investigate the depth profiles and exhibits clear signs of damage, which are discussed." @default.
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- W4210919065 date "2022-03-01" @default.
- W4210919065 modified "2023-10-02" @default.
- W4210919065 title "Raman and photoluminescence evaluation of ion-induced damage uniformity in ThO2" @default.
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- W4210919065 doi "https://doi.org/10.1016/j.nimb.2022.01.011" @default.
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