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- W4210947584 abstract "Metallic-phase selenide molybdenum (1T-MoSe2 ) has become a rising star for sodium storage in comparison with its semiconductor phase (2H-MoSe2 ) owing to the intrinsic metallic electronic conductivity and unimpeded Na+ diffusion structure. However, the thermodynamically unstable nature of 1T phase renders it an unprecedented challenge to realize its phase control and stabilization. Herein, a plasma-assisted P-doping-triggered phase-transition engineering is proposed to synthesize stabilized P-doped 1T phase MoSe2 nanoflower composites (P-1T-MoSe2 NFs). Mechanism analysis reveals significantly decreased phase-transition energy barriers of the plasma-induced Se-vacancy-rich MoSe2 from 2H to 1T owing to its low crystallinity and reduced structure stability. The vacancy-rich structure promotes highly concentrated P doping, which manipulates the electronic structure of the MoSe2 and urges its phase transition, acquiring a high transition efficiency of 91% accompanied with ultrahigh phase stability. As a result, the P-1T-MoSe2 NFs deliver an exceptional high reversible capacity of 510.8 mAh g-1 at 50 mA g-1 with no capacity fading over 1000 cycles at 5000 mA g-1 for sodium storage. The underlying mechanism of this phase-transition engineering verified by profound analysis provides informative guide for designing advanced materials for next-generation energy-storage systems." @default.
- W4210947584 created "2022-02-09" @default.
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- W4210947584 date "2022-03-01" @default.
- W4210947584 modified "2023-10-17" @default.
- W4210947584 title "Harnessing Plasma‐Assisted Doping Engineering to Stabilize Metallic Phase MoSe <sub>2</sub> for Fast and Durable Sodium‐Ion Storage" @default.
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- W4210947584 doi "https://doi.org/10.1002/adma.202200397" @default.
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