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- W4211208802 abstract "Enantioselective synthesis of axially chiral sulfur-containing biaryl derivatives through the electrophilic sulfenylation of biaryl phenols has been achieved for the first time. This catalytic asymmetric system, which involves sequential desymmetrization and kinetic resolution, is enabled by a combination of a novel 3,3'-disubstituted BINOL-derived selenide catalyst and an achiral sulfonic acid. Control experiments and computational studies suggest that multiple noncovalent interactions between the cocatalysts and substrate, especially a network of hydrogen bond interactions, play a crucial role in determining the enantioselectivity and reactivity." @default.
- W4211208802 created "2022-02-13" @default.
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- W4211208802 date "2022-02-10" @default.
- W4211208802 modified "2023-10-16" @default.
- W4211208802 title "Chiral Selenide/Achiral Sulfonic Acid Cocatalyzed Atroposelective Sulfenylation of Biaryl Phenols via a Desymmetrization/Kinetic Resolution Sequence" @default.
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- W4211208802 doi "https://doi.org/10.1021/jacs.1c09635" @default.
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