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- W4211238142 endingPage "103896" @default.
- W4211238142 startingPage "103896" @default.
- W4211238142 abstract "Although ceramic solid electrolytes, such as Li7La3Zr2O12 (LLZO), are promising candidates to replace conventional liquid electrolytes for developing safe and high-energy-density solid-state Li-metal batteries, the large interfacial resistance between cathodes and ceramic solid electrolytes severely limits their practical application. Here we developed an ionic liquid (IL)-containing while nonfluidic quasi-solid-state LiCoO2 (LCO) composite cathode, which can maintain good contact with an Al-doped LLZO (Al-LLZO) ceramic electrolyte. Accordingly the interfacial resistance between LCO and Al-LLZO was significantly decreased. Quasi-solid-state LCO/Al-LLZO/Li cells demonstrated relatively high capacity retention of about 80% after 100 cycles at 60°C. The capacity decay was mainly because of the instability of the IL. Nevertheless, the IL-containing LCO cathode enabled the use of Al-LLZO as a solid electrolyte in a simple and practical way. Identifying a suitable IL is critical for the development of quasi-solid-state Li-metal batteries with a ceramic solid electrolyte." @default.
- W4211238142 created "2022-02-13" @default.
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- W4211238142 date "2022-03-01" @default.
- W4211238142 modified "2023-09-25" @default.
- W4211238142 title "Ionic liquid-containing cathodes empowering ceramic solid electrolytes" @default.
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- W4211238142 doi "https://doi.org/10.1016/j.isci.2022.103896" @default.
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