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- W4211248155 abstract "A series of amphiphilic particles were prepared using Janus graphene oxide (GO) and magnetic SiO2-NH2 (mSiO2-NH2) as starting materials. Then, H3PW12O40 (HPW) was supported on the particles through the interaction between surface amino groups and HPW to obtain catalytic emulsion stabilizers for oxidative desulfurization. The characterization analysis showed that the prepared materials exhibited the sheet structure of GO which was connected by several core–shell microspheres of mSiO2 on one side, and the other side of the materials was grafted by carbon chains to increase hydrophobicity. The catalytic performance of prepared materials increased with the grafted carbon chain length, and the one grafted by hexadecylamine had the best performance with a final desulfurization ratio of 99.21%. That was because it had the most appropriate amphipathy, which can convert the bi-phase system into a stable Pickering emulsion with enlarged contact area between oil and extractant, thus largely promoting mass transfer even without stirring. With the excellent magnetism, the catalytic emulsion stabilizers can be magnetically separated to realize the emulsion breaking, thus easily recycling the catalyst and value-added reaction products after reaction." @default.
- W4211248155 created "2022-02-13" @default.
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- W4211248155 date "2022-05-01" @default.
- W4211248155 modified "2023-09-28" @default.
- W4211248155 title "Magnetically recyclable HPW@ mSiO2/hydrophobic GO with adjustable polarity used for oxidative desulfurization in Pickering emulsion" @default.
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- W4211248155 doi "https://doi.org/10.1016/j.fuel.2022.123239" @default.
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