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• W4211255327 abstract "Economical CO2 capture demands low-energy separation strategies. We use a liquid-infused surface (LIS) approach to immobilize reactive liquids, such as amines, on a textured and thermally conductive solid substrate with high surface-area to volume ratio (A/V) continuum geometry. The infused, micrometer-thick liquid retains that high A/V and directly contacts the gas phase, alleviating mass transport resistance typically encountered in mesoporous solid adsorbents. We name this LIS class solid with infused reactive liquid (SWIRL). SWIRL-amine requires no water dilution or costly mixing unlike the current liquid-based commercial approach. SWIRL-tetraethylenepentamine (TEPA) shows stable, high capture capacities at power plant CO2 concentrations near flue gas temperatures, preventing energy-intensive temperature swings needed for other approaches. Water vapor increases CO2 capacity of SWIRL-TEPA without compromising stability." @default.
• W4211255327 created "2022-02-13" @default.
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• W4211255327 date "2022-02-11" @default.
• W4211255327 modified "2023-10-17" @default.
• W4211255327 title "Solid with infused reactive liquid (SWIRL): A novel liquid-based separation approach for effective CO ₂ capture" @default.
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• W4211255327 doi "https://doi.org/10.1126/sciadv.abm0144" @default.
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