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- W4212781612 abstract "Herein, a Cu(I)-catalyzed enantioselective Doyle-Kirmse reaction of allenyl sulfides and α-diazoesters is reported, which provides an efficient synthetic route to enantio-enriched chiral tertiary homopropargylic sulfides. This reaction features high enantioselectivities (up to 96 % ee) and good functional group tolerance. The alkyl substituted α-diazoester has also been demonstrated as the efficient substrates in the asymmetric Doyle-Kirmse reaction. Mechanistic studies, including kinetic experiments, were conducted to gain insights into the details of the reaction pathway. The potential synthetic utility of this protocol has also been demonstrated." @default.
- W4212781612 created "2022-02-24" @default.
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- W4212781612 date "2022-03-14" @default.
- W4212781612 modified "2023-10-14" @default.
- W4212781612 title "Cu(I)/Chiral Bisoxazoline‐Catalyzed Enantioselective Doyle‐Kirmse Reaction of Allenyl Sulfides with <i>α</i>‐Diazoesters" @default.
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- W4212781612 doi "https://doi.org/10.1002/chem.202200170" @default.
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