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- W4212866857 abstract "Tailoring electron transfer dynamics across solid-liquid interfaces is fundamental to the interconversion of electrical and chemical energy. Stacking atomically thin layers with a small azimuthal misorientation to produce moiré superlattices enables the controlled engineering of electronic band structures and the formation of extremely flat electronic bands. Here, we report a strong twist-angle dependence of heterogeneous charge transfer kinetics at twisted bilayer graphene electrodes with the greatest enhancement observed near the 'magic angle' (~1.1°). This effect is driven by the angle-dependent tuning of moiré-derived flat bands that modulate electron transfer processes with the solution-phase redox couple. Combined experimental and computational analysis reveals that the variation in electrochemical activity with moiré angle is controlled by a structural relaxation of the moiré superlattice at twist angles of <2°, and 'topological defect' AA stacking regions, where flat bands are localized, produce a large anomalous local electrochemical enhancement that cannot be accounted for by the elevated local density of states alone." @default.
- W4212866857 created "2022-02-24" @default.
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- W4212866857 date "2022-02-17" @default.
- W4212866857 modified "2023-10-16" @default.
- W4212866857 title "Tunable angle-dependent electrochemistry at twisted bilayer graphene with moiré flat bands" @default.
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- W4212866857 doi "https://doi.org/10.1038/s41557-021-00865-1" @default.
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