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• W4212875172 abstract "Because of the abundance and cost effectiveness of sodium, rechargeable sodium metal batteries have been widely studied to replace current lithium-ion batteries. However, there are some critical unresolved issues including the high reactivity of sodium, an unstable solid-electrolyte interphase (SEI), and sodium dendrite formation. While several studies have been conducted to understand sodium plating/stripping processes, only a very limited number of studies have been carried out under operando conditions. We have employed operando X-ray and optical imaging techniques to understand the mechanistic behavior of Na metal plating. The morphology of sodium metal plated on a copper electrode depends strongly on the salts and solvents used in the electrolyte. The addition of a fluorine-containing additive to a carbonate-based electrolyte, NaClO4 in propylene carbonate (PC):fluoroethylene carbonate (FEC), results in uniform sodium plating processes and much more stable cycling performance, compared to NaClO4 in PC, because of the formation of a stable SEI containing NaF. A NaF layer, on top of the sodium metal, leads to a much more uniform deposition of sodium and greatly enhanced cyclability." @default.
• W4212875172 created "2022-02-24" @default.
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• W4212875172 date "2022-02-17" @default.
• W4212875172 modified "2023-10-14" @default.
• W4212875172 title "Visualization of Sodium Metal Anodes via <i>Operando</i> X-Ray and Optical Microscopy: Controlling the Morphological Evolution of Sodium Metal Plating" @default.
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• W4212875172 doi "https://doi.org/10.1021/acsami.1c24673" @default.
• W4212875172 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35175729" @default.
• W4212875172 hasPublicationYear "2022" @default.
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