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• W4212934663 abstract "Abstract To achieve carbon neutral ambition, hydrogen (H2) has recently received significant attention as a zerocarbon fuel for internal combustion engines (ICEs) across transportation sectors. As a critical element in the analysis-led design process, a hydrogen kinetic mechanism needs to be thoroughly evaluated to support the development of high-efficiency H2-ICE combustion system concepts. In this study, recently published H2 kinetic mechanisms were reviewed and down-selected for evaluations against available laboratory data in ignition delay time (IDT) and laminar flame speed (LFS) measurements. The examination was subsequently extended to high-fidelity three-dimensional (3-D) computational fluid dynamics (CFD), spark-ignited, H2 engine simulations. Discrepancies identified at engine-relevant conditions led to a kinetics tailoring campaign based on the H2 mechanism developed by Burke et al. (2012). Selected reactions identified via global sensitivity analysis were optimized under the engine-relevant pressure-temperature conditions. The reaction rate coefficients were adjusted within the experimental and theoretical uncertainty limits by adopting a Monte-Carlo sampling approach as a searching algorithm to generate candidate mechanisms. Finally, the optimized mechanism was validated sequentially from low-dimensional (0-D and 1-D) to high-fidelity 3D CFD engine simulations. Overall, the optimized H2 kinetic model led to significantly improved predictions on capturing engine in-cylinder pressure trace and heat release rate." @default.
• W4212934663 created "2022-02-24" @default.
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• W4212934663 date "2022-02-21" @default.
• W4212934663 modified "2023-10-16" @default.
• W4212934663 title "Optimizing Hydrogen Kinetics for Zero-Carbon Emission Transport Technologies" @default.
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• W4212934663 doi "https://doi.org/10.2523/iptc-22395-ms" @default.
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