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• W4212950712 abstract "New sustainable energy conversion and storage technologies are required to address the energy crisis and CO2 emission. Among various metal-CO2 batteries that utilize CO2 and offer high energy density, rechargeable Mg-CO2 batteries based on earth-abundant and safe magnesium (Mg) metal have been limited due to the lack of a compatible electrolyte, operation atmosphere, and unambiguous reaction process. Herein, the first rechargeable nonaqueous Mg-CO2 batteries have been proposed with moisture assistance in a CO2 atmosphere. These display more than 250 h cycle life and maintain the discharge voltage over 1 V at 200 mA g-1 . Combining with the experimental observations and theoretical calculations, the reaction in the moisture-assisted Mg-CO2 battery is revealed to be 2 Mg+3 CO2 +6 H2 O↔2 MgCO3 ⋅3 H2 O+C. It is anticipated that the moisture-assisted rechargeable Mg-CO2 batteries would stimulate the development of multivalent metal-CO2 batteries and extend CO2 fixation and utilization for carbon neutrality." @default.
• W4212950712 created "2022-02-24" @default.
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• W4212950712 date "2022-03-02" @default.
• W4212950712 modified "2023-10-02" @default.
• W4212950712 title "A Moisture‐Assisted Rechargeable Mg−CO₂ Battery" @default.
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• W4212950712 doi "https://doi.org/10.1002/anie.202200181" @default.
• W4212950712 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35170161" @default.
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