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- W4213126067 abstract "Abstract A state‐of‐the‐art operando spectroscopic technique is applied to Co/TiO 2 catalysts, which account for nearly half of the world's transportation fuels produced by Fischer–Tropsch catalysis. This allows determination of, at a spatial resolution of approximately 50 nm, the interdependence of formed hydrocarbon species in the inorganic catalyst. Observed trends show intra‐ and interparticular heterogeneities previously believed not to occur in particles under 200 μm. These heterogeneities are strongly dependent on changes in H 2 /CO ratio, but also on changes thereby induced on the Co and Ti valence states. We have captured the genesis of an active FTS particle over its propagation to steady‐state operation, in which microgradients lead to the gradual saturation of the Co/TiO 2 catalyst surface with long chain hydrocarbons (i.e., organic film formation)." @default.
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- W4213126067 date "2018-08-17" @default.
- W4213126067 modified "2023-09-30" @default.
- W4213126067 title "Capturing the Genesis of an Active Fischer-Tropsch Synthesis Catalyst with Operando X-ray Nanospectroscopy" @default.
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- W4213126067 doi "https://doi.org/10.1002/ange.201806354" @default.
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