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- W4213171065 abstract "Photoelectrocatalytic hydrolysis of ammonia borane (AB) is a promising technique for producing hydrogen gas (H2) in the presence of an appropriate photocatalyst under light irradiation and bias. The application of cuprous oxide on titanium dioxide nanotube arrays (Cu2O/TNA) for the photoelectrocatalytic hydrolysis of AB was studied. Cu2O/TNA exhibited a spectral response in the ultraviolet–visible region and an onset wavelength of 600 nm. With AB in an electrolyte, Cu2O/TNA exhibited a significant increase in its photocurrent spectral response at a bias of 0.1 V versus Ag/AgCl. The H2 generation rate by photoelectrocatalysis (under 5-mW cm−2 irradiation at 455 nm; bias of 0.1 V vs. Ag/AgCl) was 0.018 μmol s−1 cm−2, which was twice that by photocatalysis and four times those by catalysis and electrocatalysis; a Faradaic efficiency of 77% (corresponding to the oxidation reaction of AB) was also observed. Hence, Cu2O/TNA is an efficient photoanode for photoelectrocatalytic hydrolysis of AB." @default.
- W4213171065 created "2022-02-24" @default.
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- W4213171065 date "2022-03-01" @default.
- W4213171065 modified "2023-10-10" @default.
- W4213171065 title "Photoelectrocatalytic hydrolysis of ammonia borane by electrochemical deposited cuprous oxide on titanium dioxide nanotube arrays" @default.
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- W4213171065 doi "https://doi.org/10.1016/j.ijhydene.2022.01.167" @default.
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