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• W4213302719 endingPage "117779" @default.
• W4213302719 startingPage "117779" @default.
• W4213302719 abstract "In recent years, functional oxide-metal based vertically aligned nanocomposite (VAN) thin films have gained interest due to their intriguing physical properties and multifunctionalities stemming from the complex interactions between the two phases in the film and the substrate. In this work, we develop a model for studying the energetics of these thin film systems, including the effects of both lattice mismatch and capillary forces due to interface curvature. Each phase is incorporated into the model using a phase indicator function, and we introduce the capillary forces as body forces using a vector density representation of the interface. The model is implemented using the finite element method to study the deformation of the thin film which is composed of Au nanopillars embedded in a La0.7Sr0.3MnO3 (LSMO) matrix on an SrTiO3 (STO) substrate. The results suggest that the total energy is lowest for random configurations of pillars compared to ordered square and hexagonal lattice configurations, consistent with the random distribution of pillars found in experiments. Furthermore, we find that the interfacial energy dominates the total energy of each configuration, suggesting that interfacial energy in the system is an important design parameter for nanocomposite growth, along with the lattice mismatch." @default.
• W4213302719 created "2022-02-24" @default.
• W4213302719 creator A5000809118 @default.
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• W4213302719 date "2022-04-01" @default.
• W4213302719 modified "2023-10-03" @default.
• W4213302719 title "A generalized 3D elastic model for nanoscale, self-assembled oxide-metal thin films with pillar-in-matrix configurations" @default.
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• W4213302719 doi "https://doi.org/10.1016/j.actamat.2022.117779" @default.
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