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- W4214631741 abstract "We herein report a convenient method to convert olefins to organic iodides and amines using an Ir/ZhaoPhos catalyst, molecular hydrogen, and an electrophilic iodine(I) reagent. High yields and regioselectivities were obtained under mild conditions. In addition, basic workup with potassium carbonate leads to C-N products. Control experiments and DFT calculations tentatively excluded the pathway involving the in situ formation of HI. Instead, a catalytic cycle involving the hydrogenation of the haliranium ion intermediate was proposed." @default.
- W4214631741 created "2022-03-02" @default.
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- W4214631741 date "2022-02-24" @default.
- W4214631741 modified "2023-10-16" @default.
- W4214631741 title "Iridium-Catalyzed Hydroiodination and Formal Hydroamination of Olefins with <i>N-</i>Iodo Reagents and Molecular Hydrogen: An Umpolung Strategy" @default.
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- W4214631741 doi "https://doi.org/10.1021/acs.orglett.2c00392" @default.
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