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- W4214740762 abstract "In this study, CdSe cluster-modified biogenic α − FeOOH based on macroporous biochar was constructed from rhizosphere iron plaque via pyrolysis. An ultrahigh H2O2 production rate of 655.75 μmol/L was achieved by the photocatalysis-self-Fenton system within 30 min under visible light irradiation. α-FeOOH, with abundant iron ions, can directly activate H2O2 to produce abundant ⋅OH radicals. It was found that As(III) (10 mg/L) could be completely degraded within 20 min. Electron spin resonance spectroscopy (ESR) and density functional theory (DFT) revealed that a suitable energy band structure was achieved by the introduction of CdSe clusters; thus, O2 was mainly reduced to H2O2 through a two-electron reduction route in the reaction system. The photogenerated electrons promoted the conversion of Fe(III)/Fe(II) by reacting with Fe(III) in α-FeOOH. The presence of H2O2 and Fe2+ in this system accelerates the oxidation of As(III) by a Fenton-like reaction." @default.
- W4214740762 created "2022-03-02" @default.
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- W4214740762 date "2022-07-01" @default.
- W4214740762 modified "2023-09-30" @default.
- W4214740762 title "CdSe cluster-modified biogenic α-FeOOH based on macroporous biochar for Fenton-like reaction of As(III)" @default.
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- W4214740762 doi "https://doi.org/10.1016/j.apsusc.2022.152872" @default.
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