Matches in SemOpenAlex for { <https://semopenalex.org/work/W4220659191> ?p ?o ?g. }
- W4220659191 abstract "Abstract Surface chemistry mediated direct optical patterning represents an emerging strategy for incorporating colloidal nanocrystals (NCs) in integrated optoelectronic platforms including displays and image sensors. However, the role of photochemistry of crosslinkers and other photoactive species in patterning remains elusive. Here we show the design of nitrene‐ and carbene‐based photocrosslinkers can strongly affect the patterning capabilities and photophysical properties of NCs, especially quantum dots (QDs). Their role beyond physical linkers stems from structure‐dictated electronic configuration, energy alignment and associated reaction kinetics and thermodynamics. Patterned QD layers with designed carbene‐based crosslinkers fully preserve their photoluminescent and electroluminescent properties. Patterned light emitting diodes (QLEDs) show a maximum external quantum efficiency of ≈12 % and lifetime over 4800 h, among the highest for reported patterned QLEDs. These results would guide the rational design of photoactive species in NC patterning and create new possibilities in the monolithic integration of NCs in high‐performance device platforms." @default.
- W4220659191 created "2022-04-03" @default.
- W4220659191 creator A5001812456 @default.
- W4220659191 creator A5004086293 @default.
- W4220659191 creator A5006012404 @default.
- W4220659191 creator A5007371177 @default.
- W4220659191 creator A5022859032 @default.
- W4220659191 creator A5023574563 @default.
- W4220659191 creator A5034171151 @default.
- W4220659191 creator A5040568467 @default.
- W4220659191 creator A5040874408 @default.
- W4220659191 creator A5045019697 @default.
- W4220659191 creator A5049341927 @default.
- W4220659191 creator A5049991161 @default.
- W4220659191 creator A5052895667 @default.
- W4220659191 creator A5063331443 @default.
- W4220659191 creator A5071304644 @default.
- W4220659191 creator A5072620133 @default.
- W4220659191 creator A5076495171 @default.
- W4220659191 creator A5089448918 @default.
- W4220659191 creator A5090109818 @default.
- W4220659191 creator A5091784924 @default.
- W4220659191 date "2022-04-05" @default.
- W4220659191 modified "2023-10-18" @default.
- W4220659191 title "Beyond a Linker: The Role of Photochemistry of Crosslinkers in the Direct Optical Patterning of Colloidal Nanocrystals" @default.
- W4220659191 cites W1808639415 @default.
- W4220659191 cites W1921964650 @default.
- W4220659191 cites W1930282399 @default.
- W4220659191 cites W1973504871 @default.
- W4220659191 cites W1982827781 @default.
- W4220659191 cites W2007156945 @default.
- W4220659191 cites W2008196603 @default.
- W4220659191 cites W2013518047 @default.
- W4220659191 cites W2038602088 @default.
- W4220659191 cites W2057263316 @default.
- W4220659191 cites W2060518499 @default.
- W4220659191 cites W2065706045 @default.
- W4220659191 cites W2076418712 @default.
- W4220659191 cites W2138463916 @default.
- W4220659191 cites W2146928336 @default.
- W4220659191 cites W2173925994 @default.
- W4220659191 cites W2255871307 @default.
- W4220659191 cites W2262464189 @default.
- W4220659191 cites W2316217490 @default.
- W4220659191 cites W2322254936 @default.
- W4220659191 cites W2326153055 @default.
- W4220659191 cites W2418427990 @default.
- W4220659191 cites W2518050598 @default.
- W4220659191 cites W2531211553 @default.
- W4220659191 cites W2588217511 @default.
- W4220659191 cites W2739651090 @default.
- W4220659191 cites W2771381738 @default.
- W4220659191 cites W2890052713 @default.
- W4220659191 cites W2891484817 @default.
- W4220659191 cites W2900583170 @default.
- W4220659191 cites W2950007144 @default.
- W4220659191 cites W2951646711 @default.
- W4220659191 cites W2980068597 @default.
- W4220659191 cites W2984253303 @default.
- W4220659191 cites W3000171270 @default.
- W4220659191 cites W3014476880 @default.
- W4220659191 cites W3033478592 @default.
- W4220659191 cites W3090498325 @default.
- W4220659191 cites W3110399748 @default.
- W4220659191 cites W3119125141 @default.
- W4220659191 cites W3124705158 @default.
- W4220659191 cites W3127018183 @default.
- W4220659191 cites W3173205213 @default.
- W4220659191 cites W3183353435 @default.
- W4220659191 cites W3188217743 @default.
- W4220659191 cites W3188401157 @default.
- W4220659191 cites W3191171424 @default.
- W4220659191 cites W3193214518 @default.
- W4220659191 cites W4249916559 @default.
- W4220659191 doi "https://doi.org/10.1002/ange.202202633" @default.
- W4220659191 hasPublicationYear "2022" @default.
- W4220659191 type Work @default.
- W4220659191 citedByCount "1" @default.
- W4220659191 countsByYear W42206591912023 @default.
- W4220659191 crossrefType "journal-article" @default.
- W4220659191 hasAuthorship W4220659191A5001812456 @default.
- W4220659191 hasAuthorship W4220659191A5004086293 @default.
- W4220659191 hasAuthorship W4220659191A5006012404 @default.
- W4220659191 hasAuthorship W4220659191A5007371177 @default.
- W4220659191 hasAuthorship W4220659191A5022859032 @default.
- W4220659191 hasAuthorship W4220659191A5023574563 @default.
- W4220659191 hasAuthorship W4220659191A5034171151 @default.
- W4220659191 hasAuthorship W4220659191A5040568467 @default.
- W4220659191 hasAuthorship W4220659191A5040874408 @default.
- W4220659191 hasAuthorship W4220659191A5045019697 @default.
- W4220659191 hasAuthorship W4220659191A5049341927 @default.
- W4220659191 hasAuthorship W4220659191A5049991161 @default.
- W4220659191 hasAuthorship W4220659191A5052895667 @default.
- W4220659191 hasAuthorship W4220659191A5063331443 @default.
- W4220659191 hasAuthorship W4220659191A5071304644 @default.
- W4220659191 hasAuthorship W4220659191A5072620133 @default.
- W4220659191 hasAuthorship W4220659191A5076495171 @default.
- W4220659191 hasAuthorship W4220659191A5089448918 @default.
- W4220659191 hasAuthorship W4220659191A5090109818 @default.
- W4220659191 hasAuthorship W4220659191A5091784924 @default.