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• W4220736025 abstract "• High nitrogen content boron-containing BTDB anion was successfully synthesized. • High density-specific impulse of BTDB anion-based HILs were obtained. • DFT were illustrated the difference between the [bis(triazolyl)–BH 2 ] − anions. • Short ID time and well physico-chemical property made them suitable for propellent. As a new generation of potential rocket fuel, hypergolic ionic liquids, especially boron-containing hypergolic ionic liquids, have emerged as attractive alternatives for unsymmetrical dimethylhydrazine (UDMH). Herein, a series of bis(1H-1,2,3-triazole-1-yl) dihydroborate (BTDB) hypergolic ionic liquids were successfully synthesized, which had a melting point below -60 °C, high density ranging from 1.134 g/cm 3 to 1.173 g/cm 3 , and superior density-specific impulse from 374.2 to 386.5 s g/cm 3 . In particular, 1,3-diallyl-1H-imidazol-3-ium bis(1H-1,2,3-triazole-1-yl) dihydroborate owned an ignition-delay time of 36 ms and the enthalpy of formation about 1.78 kJ/g, exhibiting that it was a good potential for the rocket fuels. A new type of the high nitrogen content boron-containing di(1H-1,2,3-triazole-1-yl)dihydroborate anion was successfully synthesized and demonstrated by the single crystal analysis, which could be the alternative for the hydrazines that are prone to serious pollution. Then, based on the di(1H-1,2,3-triazole-1-yl)dihydroborate anion, a series of di(1H-1,2,3-triazole-1-yl)dihydroborate hypergolic ionic liquids were prepared, which own melting points below -60 °C, a high density ranging from 1.134 g/cm 3 to 1.173 g/cm 3 , superior performance of the density-specific impulse from 374.2 to 386.5 s g/cm 3 . In particular, 1,3-diallyl-1H-imidazol-3-ium di(1H-1,2,3-triazole-1-yl)dihydroborate own an low ignition-delay time (36 ms), a high value of the enthalpies of formation (2.08 kJ/g), which shown good potential for the rocket fuels A new type of the high nitrogen content boron-containing di(1H-1,2,3-triazole-1-yl)dihydroborate anion was successfully synthesized and demonstrated by the single crystal analysis, which could be the alternative for the hydrazines that are prone to serious pollution. Then, based on the di(1H-1,2,3-triazole-1-yl)dihydroborate anion, a series of di(1H-1,2,3-triazole-1-yl)dihydroborate hypergolic ionic liquids were prepared, which own melting points below -60 °C, a high density ranging from 1.134 g/cm 3 to 1.173 g/cm 3 , superior performance of the density-specific impulse from 374.2 to 386.5 s g/cm 3 . In particular, 1,3-diallyl-1H-imidazol-3-ium di(1H-1,2,3-triazole-1-yl)dihydroborate own an low ignition-delay time (36 ms), a high value of the enthalpies of formation (2.08 kJ/g), which shown good potential for the rocket fuels." @default.
• W4220736025 created "2022-04-03" @default.
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• W4220736025 date "2022-08-01" @default.
• W4220736025 modified "2023-09-26" @default.
• W4220736025 title "Synthesis and characterization of hypergolic salts based on bis(1H-1,2,3-triazole-1-yl) dihydroborate anion" @default.
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• W4220736025 doi "https://doi.org/10.1016/j.molstruc.2022.132850" @default.
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