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• W4220740028 endingPage "1888" @default.
• W4220740028 startingPage "1883" @default.
• W4220740028 abstract "A facile synthetic method for 4-aryl-4,5-dihydropyrrole-3-carboxylates is developed, with a rhodium-catalyzed ring expansion strategy from readily available 2-(azetidin-3-ylidene) acetates and aryl boronic acids. Mechanistic investigations suggest a novel domino conjugate addition/N-directed α-C(sp3)-H activation process. The asymmetric catalytic synthesis of the 4-aryl-4,5-dihydropyrrole-3-carboxylate is realized by using QuinoxP* (91-97% ee). The synthetic utility of this protocol is demonstrated by the synthesis of 3,4-disubstituted or 2,3,4-trisubstituted pyrrolidines with excellent diastereoselectivities." @default.
• W4220740028 created "2022-04-03" @default.
• W4220740028 creator A5033398209 @default.
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• W4220740028 date "2022-03-10" @default.
• W4220740028 modified "2023-09-26" @default.
• W4220740028 title "Rhodium-Catalyzed Ring Expansion of Azetidines via Domino Conjugate Addition/N-Directed α-C(sp³)–H Activation" @default.
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• W4220740028 doi "https://doi.org/10.1021/acs.orglett.2c00056" @default.
• W4220740028 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35266389" @default.
• W4220740028 hasPublicationYear "2022" @default.
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