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• W4220776257 abstract "Employing high-voltage Ni-rich cathodes in Li metal batteries (LMBs) requires stabilization of the electrode/electrolyte interfaces at both electrodes. A stable solid-electrolyte interphase (SEI) and suppression of active material pulverization remain the greatest challenges to achieving efficient long-term cycling. Herein, studies of NMC622 (1 mAh cm-2) cathodes were performed using highly concentrated N-methyl-N-propylpyrrolidinium bis(fluorosulfonyl)imide (C3mpyrFSI) 50 mol % lithium bis(fluorosulfonyl)imide (LiFSI) ionic liquid electrolyte (ILE). The resulting SEI formed at the cathode enabled promising cycling performance (98.13% capacity retention after 100 cycles), and a low degree of ion mixing and lattice expansion was observed, even at an elevated temperature of 50 °C. Fitting of acquired impedance spectra indicated that the SEI resistivity (RSEI) had a low and stable contribution to the internal resistivity of the system, whereas active material pulverization and secondary grain isolation significantly increased the charge transfer resistance (RCT) throughout cycling." @default.
• W4220776257 created "2022-04-03" @default.
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• W4220776257 date "2022-03-11" @default.
• W4220776257 modified "2023-10-16" @default.
• W4220776257 title "Morphological Evolution and Solid–Electrolyte Interphase Formation on LiNi_0.6Mn_0.2Co_0.2O₂ Cathodes Using Highly Concentrated Ionic Liquid Electrolytes" @default.
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• W4220776257 doi "https://doi.org/10.1021/acsami.1c21853" @default.
• W4220776257 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35274926" @default.
• W4220776257 hasPublicationYear "2022" @default.
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