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- W4220776882 abstract "• Supramolecular eutectogels show rapid self-healing ability and excellent mechanical strength. • Supramolecular eutectogels exhibits good load-bearing capacity and injectability. • Supramolecular eutectogels can be applied to smart conductive materials, interface lubrication and dye adsorption. The self-healing eutectogels with multifunctionality have attracted much attention in soft materials owing to their high conductivity and non-volatility. However, obtaining eutectogels with complete recovery of mechanical properties is still challenging. Herein, we developed a series of halogenated dibenzylidene-D-sorbitol (X-DBS) gelators. The X-DBS could form eutectogels in deep eutectic solvents obtained from choline chloride combined with alcohols or urea, which exhibit self-healing, complete recovery, load-bearing, and injectability. Fourier transform infrared, 19 F nuclear magnetic resonance, and molecular dynamics simulations showed that the hydrogen bond between the C-F bond and the solvent molecule is key to the self-healing property of the eutectogels. Interestingly, the high ionic conductivity and self-healing property of our eutectogel make it potentially useful in a smart ionic conductor. Moreover, the self-healing eutectogels with corrosion resistance showed good lubricating performances on steel interfaces. In addition, the eutectogels showed excellent dye adsorption, effectively removing dyes from aqueous solutions. Thus, the efficient DBS-based eutectogels with self-healing properties are excellent candidates for conductive materials, interfacial lubrication, dye adsorption, and other applications." @default.
- W4220776882 created "2022-04-03" @default.
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- W4220776882 date "2022-08-01" @default.
- W4220776882 modified "2023-10-16" @default.
- W4220776882 title "Multifunctional self-healing eutectogels induced by supramolecular assembly for smart conductive materials, interface lubrication and dye adsorption" @default.
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- W4220776882 doi "https://doi.org/10.1016/j.cej.2022.136026" @default.
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