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- W4220781502 abstract "To develop simple catalytic systems without well-defined tertiary structures is of paramount importance to perform bio-inspired chemistry but remains challenge. Here, we have developed a simple one-step strategy for preparing polystyrene-supported artificial catalytic triad (ACT) systems. Polymers containing ACTs and a polymer containing urea groups were designed and synthesized for the preparation of catalysts via nanoprecipitation. The coil-globule collapse of polystyrene chains created hydrophobic microenvironments. The catalytic performance could be regulated by altering polymer compositions. The hydrophobic microenvironments played important roles in the efficiency of polystyrene-supported artificial catalytic triads, arising from varied affinity for the hydrophobic substrates and/or regulating the local pKa of artificial catalytic triads. A postulated mechanism for ester hydrolysis over polystyrene-supported catalysts was presented. This strategy has potential applications for engineering other multifunctional, enzyme-inspired catalysts." @default.
- W4220781502 created "2022-04-03" @default.
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- W4220781502 date "2022-07-01" @default.
- W4220781502 modified "2023-10-14" @default.
- W4220781502 title "Engineering of polystyrene-supported artificial catalytic triad constructed by nanoprecipitation for efficient ester hydrolysis in water" @default.
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- W4220781502 doi "https://doi.org/10.1016/j.colsurfa.2022.128902" @default.
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