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• W4220783411 abstract "This manuscript describes a universal method for the spontaneous self-assembly of nanostructures ranging from 2-4 nm spherical particles to ∼440 nm long anisotropic nanorods into ring-like superstructures. The nanostructures composed of Au, Pt, and Pd as surface materials were synthesized in an aqueous cetyltrimethyl ammonium bromide (CTAB) solution. The ligand exchange technique with 4-mercaptophenol was applied to replace CTAB from the surface of nanostructures with a functional thiol. The esterification reaction was carried out to covalently attach carboxy-terminated long-chain polystyrene (PS) molecules to the surface of nanostructures. The high grafting density of PS chains around nanocrystals made them highly soluble in a wide range of organic solvents. When a drop of nanostructure solution in a volatile nonpolar solvent was dried on a solid surface, the nanostructures spontaneously arranged themselves in the form of ring-like assemblies. The condensation of microscopic water droplets from the atmosphere on the surface of an evaporating solvent creates templates for the self-assembly of nanostructures into rings. We demonstrate that this self-assembly method is highly universal and can be extended to various nanostructures regardless of their shapes, sizes, and surface materials." @default.
• W4220783411 created "2022-04-03" @default.
• W4220783411 creator A5007194666 @default.
• W4220783411 creator A5072534261 @default.
• W4220783411 date "2022-03-17" @default.
• W4220783411 modified "2023-09-27" @default.
• W4220783411 title "Self-Assembly of Nanocrystals into Ring-like Superstructures: When Shape, Size, and Material Do Not Matter" @default.
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• W4220783411 doi "https://doi.org/10.1021/acs.langmuir.2c00153" @default.
• W4220783411 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35298173" @default.
• W4220783411 hasPublicationYear "2022" @default.
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