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- W4220792695 abstract "Abstract Disclosed herein is a photoinduced selective hydroamination of ynamides with nitrogen heteroaromatic nucleophiles. By using an organocatalytic photoredox system, a direct method to construct a diverse of ( Z )‐α‐azole enamides from ynamides and pyrazoles, as well as triazoles, benzotriazoles, indazoles, and tetrazoles, is developed, thus providing a photocatalytically synthetic route to heterocyclic motifs common in medicinal agents. Based on the mechanistic studies, the hydroamination is postulated to operate via a mechanism in which the single‐electron oxidation of ynamide and the intermediacy of an alkyne radical cation, is responsible for the observed reactivity. magnified image" @default.
- W4220792695 created "2022-04-03" @default.
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- W4220792695 date "2022-02-03" @default.
- W4220792695 modified "2023-09-26" @default.
- W4220792695 title "Organic Photoredox Catalyzed Direct Hydroamination of Ynamides with Azoles" @default.
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- W4220792695 doi "https://doi.org/10.1002/adsc.202101410" @default.
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