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• W4220793908 endingPage "121352" @default.
• W4220793908 startingPage "121352" @default.
• W4220793908 abstract "The sluggish kinetics of oxygen electrode reactions is a bottleneck for the development of rechargeable Zn-air batteries (ZABs). Herein, we report a bifunctional electrocatalyst synthesized by anchoring individually dispersed Ni single atoms on N-doped carbon nanosheets (Ni SAs-NC), which exhibits an outstanding overall performance for oxygen reduction reaction (ORR) and urea oxidation reaction (UOR). Based on that, a conceptual urea-assisted rechargeable ZAB by coupling ORR with UOR of a low thermodynamic potential is demonstrated to have significantly decreased charging voltage and high urea elimination rate. The high bifunctional electrocatalytic activities of Ni SAs-NC endow the urea-assisted ZAB with a dramatically increased energy conversion efficiency of 71.8%, which is improved by 17.1% as compares with the conventional ZABs. The successful implementation of Ni SACs based urea-assisted rechargeable ZABs with an improved energy conversion efficiency may prompt ZAB technology towards practical applications." @default.
• W4220793908 created "2022-04-03" @default.
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• W4220793908 date "2022-08-01" @default.
• W4220793908 modified "2023-10-13" @default.
• W4220793908 title "Ni single atoms anchored on N-doped carbon nanosheets as bifunctional electrocatalysts for Urea-assisted rechargeable Zn-air batteries" @default.
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• W4220793908 doi "https://doi.org/10.1016/j.apcatb.2022.121352" @default.
• W4220793908 hasPublicationYear "2022" @default.
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