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• W4220795411 abstract "Dry reforming of methane (DRM) has provided an effective avenue to convert two greenhouse gases, CH4 and CO2 , into syngas. Here, we design a DRM photocatalyst Rh/Cex WO3 that invokes both photothermal and photoelectric processes, which overcomes the thermodynamic limitation of DRM under conventional conditions. In contrast to plasmonic or UV-response photocatalysts, our photocatalyst produces a superior light-to-chemical energy efficiency (LTCEE) of 4.65 % with a moderate light intensity. We propose that a light-induced metal-to-metal charge transfer plays a crucial role in the DRM reaction, which induces a redox looping between Ce to W species to lower the activation energy. Quantum mechanical studies reveal that a high oxygen mobility of Cex WO3 , accompanied with the formation of oxo-bridge species, results in a substantial elimination of deposited C species during the reaction. Our catalyst design strategy could offer a promising energy-efficient industrial process for DRM." @default.
• W4220795411 created "2022-04-03" @default.
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• W4220795411 date "2022-03-23" @default.
• W4220795411 modified "2023-10-03" @default.
• W4220795411 title "Light‐Induced Redox Looping of a Rhodium/Ce _<i>x</i> WO ₃ Photocatalyst for Highly Active and Robust Dry Reforming of Methane" @default.
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• W4220795411 doi "https://doi.org/10.1002/anie.202200567" @default.
• W4220795411 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35277912" @default.
• W4220795411 hasPublicationYear "2022" @default.
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