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- W4220802973 abstract "A novel material with N-doped carbon dots decorated three-dimensional graphitic carbon nitride (NCDs/TCN) is synthesized using NaCl as template. Abundant Na+ are found to be in-situ doped in 3D g-C3N4 framework. Experiments and density functional theory (DFT) calculations suggest that peroxydisulfate (PDS) activation follows radical and non-radical pathways on the NCDs/TCN catalyst. NCDs have superior up-conversion photoluminescence property and can enhance charge separation efficiency, thus improving the photocatalytic reactivity of 3D g-C3N4 and promoting the radical activation of PDS efficiently. Interestingly, the NCDs/TCN-PDS* complex can be formed due to the large adsorption energy of doped Na+ for PDS, thus inducing the non-radical PDS activation pathway. This work provides an effective approach to combine radical and non-radical pathways for boosting PDS activation and gives deep insights for the non-radical pathway induced by doped Na+ in 3D g-C3N4." @default.
- W4220802973 created "2022-04-03" @default.
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- W4220802973 date "2022-08-01" @default.
- W4220802973 modified "2023-09-30" @default.
- W4220802973 title "N-doped carbon dots decorated 3D g-C3N4 for visible-light driven peroxydisulfate activation: Insights of non-radical route induced by Na+ doping" @default.
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- W4220802973 doi "https://doi.org/10.1016/j.apcatb.2022.121304" @default.
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