FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4220876017> ?p ?o ?g. }

• W4220876017 endingPage "128796" @default.
• W4220876017 startingPage "128796" @default.
• W4220876017 abstract "Black TiO2 nanotube arrays (black TNAs) suffer from the low activity and deactivation for peroxymonosulfate (PMS) activation, which limit their application in the oxidative destruction of organic pollutants in water. Here, we report an efficient, environmentally benign, and cost-effective method to enhance the catalytic activity and prevent the deactivation of black TNAs in PMS activation by utilizing solar energy. Optical absorption and electrochemical analysis and density functional theory calculations demonstrated that abundant oxygen vacancies (estimated to be 26%) on the black TNAs surface markedly improved solar light absorption and electrical conductivity and played a critical role as a catalytic active site for PMS activation. As a result, the solar light-irradiated black TNAs/PMS system exhibited the higher phenol degradation rate (k = 0.0488 min-1) and total organic carbon (TOC) removal efficiency (~70%) compared to other TNAs systems. These results were ascribed to the switching of the reaction mechanism from non-radical mechanism to radical-involved. Black TNAs oxidized organic pollutants by mediating electron transfer from organics to PMS in the dark (i.e., a non-radical pathway). On the other hand, PMS activation under solar light irradiation involved the production of highly reactive sulfate and hydroxyl radicals (i.e., radical pathway), markedly improving the degradation and mineralization of organics. Additionally, the solar light-irradiated black TNAs showed relative pH-independence for PMS activation and durable catalytic performance without the loss of activity during the repetitive reaction cycles." @default.
• W4220876017 created "2022-04-03" @default.
• W4220876017 creator A5012389196 @default.
• W4220876017 creator A5028246371 @default.
• W4220876017 creator A5072346189 @default.
• W4220876017 creator A5084241485 @default.
• W4220876017 date "2022-07-01" @default.
• W4220876017 modified "2023-10-13" @default.
• W4220876017 title "Peroxymonosulfate activation by black TiO2 nanotube arrays under solar light: Switching the activation mechanism and enhancing catalytic activity and stability" @default.
• W4220876017 cites W1918325227 @default.
• W4220876017 cites W1926950498 @default.
• W4220876017 cites W1970127494 @default.
• W4220876017 cites W1973231138 @default.
• W4220876017 cites W1978422337 @default.
• W4220876017 cites W1981368803 @default.
• W4220876017 cites W1982187838 @default.
• W4220876017 cites W1991695524 @default.
• W4220876017 cites W2006060524 @default.
• W4220876017 cites W2007544004 @default.
• W4220876017 cites W2027244517 @default.
• W4220876017 cites W2031283815 @default.
• W4220876017 cites W2032578873 @default.
• W4220876017 cites W2038132462 @default.
• W4220876017 cites W2038805521 @default.
• W4220876017 cites W2052452584 @default.
• W4220876017 cites W2061217425 @default.
• W4220876017 cites W2079253547 @default.
• W4220876017 cites W2081709688 @default.
• W4220876017 cites W2083222334 @default.
• W4220876017 cites W2091002202 @default.
• W4220876017 cites W2096747776 @default.
• W4220876017 cites W2102901965 @default.
• W4220876017 cites W2109325117 @default.
• W4220876017 cites W2166828764 @default.
• W4220876017 cites W2275668394 @default.
• W4220876017 cites W2294653078 @default.
• W4220876017 cites W2320148161 @default.
• W4220876017 cites W2330618834 @default.
• W4220876017 cites W2333946702 @default.
• W4220876017 cites W2509538092 @default.
• W4220876017 cites W2513165742 @default.
• W4220876017 cites W2523737452 @default.
• W4220876017 cites W2534737939 @default.
• W4220876017 cites W2581655244 @default.
• W4220876017 cites W2608529282 @default.
• W4220876017 cites W2610959597 @default.
• W4220876017 cites W2763540983 @default.
• W4220876017 cites W2765231708 @default.
• W4220876017 cites W2770125280 @default.
• W4220876017 cites W2772029075 @default.
• W4220876017 cites W2786783287 @default.
• W4220876017 cites W2789196588 @default.
• W4220876017 cites W2792221401 @default.
• W4220876017 cites W2793349440 @default.
• W4220876017 cites W2798227067 @default.
• W4220876017 cites W2799501583 @default.
• W4220876017 cites W2945424499 @default.
• W4220876017 cites W2979903809 @default.
• W4220876017 cites W2981353654 @default.
• W4220876017 cites W2984564882 @default.
• W4220876017 cites W2985585673 @default.
• W4220876017 cites W3037790339 @default.
• W4220876017 cites W3044499469 @default.
• W4220876017 cites W3048371319 @default.
• W4220876017 cites W3097347296 @default.
• W4220876017 cites W3101719451 @default.
• W4220876017 cites W3109305436 @default.
• W4220876017 cites W3120204822 @default.
• W4220876017 cites W3121064953 @default.
• W4220876017 cites W3184197505 @default.
• W4220876017 cites W3211760050 @default.
• W4220876017 doi "https://doi.org/10.1016/j.jhazmat.2022.128796" @default.
• W4220876017 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35366445" @default.
• W4220876017 hasPublicationYear "2022" @default.
• W4220876017 type Work @default.
• W4220876017 citedByCount "17" @default.
• W4220876017 countsByYear W42208760172022 @default.
• W4220876017 countsByYear W42208760172023 @default.
• W4220876017 crossrefType "journal-article" @default.
• W4220876017 hasAuthorship W4220876017A5012389196 @default.
• W4220876017 hasAuthorship W4220876017A5028246371 @default.
• W4220876017 hasAuthorship W4220876017A5072346189 @default.
• W4220876017 hasAuthorship W4220876017A5084241485 @default.
• W4220876017 hasConcept C127413603 @default.
• W4220876017 hasConcept C139066938 @default.
• W4220876017 hasConcept C161790260 @default.
• W4220876017 hasConcept C176933379 @default.
• W4220876017 hasConcept C178790620 @default.
• W4220876017 hasConcept C185592680 @default.
• W4220876017 hasConcept C2776778087 @default.
• W4220876017 hasConcept C42360764 @default.
• W4220876017 hasConcept C44038986 @default.
• W4220876017 hasConcept C75473681 @default.
• W4220876017 hasConcept C95121573 @default.
• W4220876017 hasConceptScore W4220876017C127413603 @default.
• W4220876017 hasConceptScore W4220876017C139066938 @default.
• W4220876017 hasConceptScore W4220876017C161790260 @default.
• W4220876017 hasConceptScore W4220876017C176933379 @default.

• next