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- W4220893266 abstract "Abstract The state with effective total moment J eff = 1/2 stabilized by the spin-orbit coupling is known to suppress Jahn-Teller distortions and may induce a strong exchange anisotropy. This in turn may lead to the formation of an elusive spin-liquid state in real materials. While recent studies have demonstrated that such a situation can be realized in 3 d transition-metal compounds such as those based on Co 2+ and Cu 2+ , diagnosis of J eff = 1/2 state remains challenging. We show that resonant inelastic X-ray scattering is an effective tool to probe this state and apply it to CuAl 2 O 4 , material where Cu 2+ ions were previously proposed to be in the J eff = 1/2 state. Our results unambiguously demonstrate that, contrary to previous expectations, a competitive (to J eff = 1/2) Jahn-Teller state realizes in this compound." @default.
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- W4220893266 date "2022-03-21" @default.
- W4220893266 modified "2023-10-17" @default.
- W4220893266 title "Resonant inelastic X-ray scattering as a probe of Jeff = 1/2 state in 3d transition-metal oxide" @default.
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- W4220893266 doi "https://doi.org/10.1038/s41535-022-00430-0" @default.
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