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- W4220948632 abstract "Mechanically strengthened fiber-supercapacitors (FSCs) are urgently needed in wearable electronics to adapt frequent severe deformations. However, current bendable FSCs using gel electrolyte as separator are easily short-circuited under harsh folding due to the limited stretchability of gel polymer. Herein, a folding-resistant coaxial FSC, for the first time, was fabricated through in-situ electrospinning polyacrylonitrile (PAN) nanofibers as separator on fiber electrode, thus effectively avoiding the short-circuit risk under highly localized stretching, compressing and folding. Moreover, such “epitaxial growth” ultrathin (∼ 1 µm) PAN separator possesses high porosity, favorable strength and seamless contact with fiber electrode, enabling fast ion transport and decreased internal resistance of FSCs. Coupled with robust polyaniline/carbon nanotube (PANI/CNT) composite as model electrodes, our fabricated coaxial symmetric FSC exhibits outstanding structural folding-resistance without electrochemical failure. Amazingly, such in-situ encapsulated separator technique makes it easier to assemble multi-layer PANI/CNT electrode in series or parallel. As-assembled coaxial integrated series or parallel device keeps almost same volume as single device, but delivers higher output voltage or capacitance; and simultaneously remains excellent foldable property, showing great practical potential." @default.
- W4220948632 created "2022-04-03" @default.
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- W4220948632 date "2022-08-01" @default.
- W4220948632 modified "2023-10-15" @default.
- W4220948632 title "Epitaxial nanofiber separator enabling folding-resistant coaxial fiber-supercapacitor module" @default.
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- W4220948632 doi "https://doi.org/10.1016/j.ensm.2022.03.011" @default.
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