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• W4220971304 abstract "We report a Pd-catalyzed route to heterocycles bearing a tetrasubstituted alkene fragment. Our approach merges the intramolecular carbopalladation of tethered alkynes with an alkylation step produced by the C-C cleavage of cyclobutanol derivatives. An alkenyl-Pd(II) intermediate has been isolated and characterized by X-ray diffraction studies. Interestingly, the nature of the tethering alkynyl chain influences the E/Z stereochemistry of the alkenyl fragment in the functionalized heterocycles." @default.
• W4220971304 created "2022-04-03" @default.
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• W4220971304 date "2022-03-03" @default.
• W4220971304 modified "2023-10-18" @default.
• W4220971304 title "Synthesis of Benzofused <i>O</i>- and <i>N</i>-Heterocycles through Cascade Carbopalladation/Cross-Alkylation of Alkynes Involving the C–C Cleavage of Cyclobutanols" @default.
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• W4220971304 doi "https://doi.org/10.1021/acs.organomet.2c00015" @default.
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