Matches in SemOpenAlex for { <https://semopenalex.org/work/W4220971757> ?p ?o ?g. }
- W4220971757 abstract "Abstract Catalytic solvent regeneration has attracted broad interest owing to its potential to reduce energy consumption in CO 2 separation, enabling industry to achieve emission reduction targets of the Paris Climate Accord. Despite recent advances, the development of engineered acidic nanocatalysts with unique characteristics remains a challenge. Herein, we establish a strategy to tailor the physicochemical properties of metal-organic frameworks (MOFs) for the synthesis of water-dispersible core-shell nanocatalysts with ease of use. We demonstrate that functionalized nanoclusters (Fe 3 O 4 -COOH) effectively induce missing-linker deficiencies and fabricate mesoporosity during the self-assembly of MOFs. Superacid sites are created by introducing chelating sulfates on the uncoordinated metal clusters, providing high proton donation capability. The obtained nanomaterials drastically reduce the energy consumption of CO 2 capture by 44.7% using only 0.1 wt.% nanocatalyst, which is a ∽10-fold improvement in efficiency compared to heterogeneous catalysts. This research represents a new avenue for the next generation of advanced nanomaterials in catalytic solvent regeneration." @default.
- W4220971757 created "2022-04-03" @default.
- W4220971757 creator A5010731144 @default.
- W4220971757 creator A5012386870 @default.
- W4220971757 creator A5014874162 @default.
- W4220971757 creator A5022785909 @default.
- W4220971757 creator A5031877516 @default.
- W4220971757 creator A5050500604 @default.
- W4220971757 creator A5068761476 @default.
- W4220971757 creator A5073206123 @default.
- W4220971757 creator A5076923063 @default.
- W4220971757 creator A5091386340 @default.
- W4220971757 date "2022-03-10" @default.
- W4220971757 modified "2023-10-10" @default.
- W4220971757 title "Engineered assembly of water-dispersible nanocatalysts enables low-cost and green CO2 capture" @default.
- W4220971757 cites W1065539523 @default.
- W4220971757 cites W1973993234 @default.
- W4220971757 cites W1986238480 @default.
- W4220971757 cites W2015723183 @default.
- W4220971757 cites W2106070699 @default.
- W4220971757 cites W2130579587 @default.
- W4220971757 cites W2153201248 @default.
- W4220971757 cites W2412540263 @default.
- W4220971757 cites W2617021599 @default.
- W4220971757 cites W2696171370 @default.
- W4220971757 cites W2767662331 @default.
- W4220971757 cites W2799696644 @default.
- W4220971757 cites W2810755092 @default.
- W4220971757 cites W2883884681 @default.
- W4220971757 cites W2888488148 @default.
- W4220971757 cites W2899810052 @default.
- W4220971757 cites W2941498316 @default.
- W4220971757 cites W2943791925 @default.
- W4220971757 cites W2947643484 @default.
- W4220971757 cites W2947781114 @default.
- W4220971757 cites W2954591269 @default.
- W4220971757 cites W2964314984 @default.
- W4220971757 cites W2966060513 @default.
- W4220971757 cites W2969453684 @default.
- W4220971757 cites W2975696614 @default.
- W4220971757 cites W2979795026 @default.
- W4220971757 cites W2992462999 @default.
- W4220971757 cites W2998402750 @default.
- W4220971757 cites W3016104265 @default.
- W4220971757 cites W3019024674 @default.
- W4220971757 cites W3023124676 @default.
- W4220971757 cites W3028678034 @default.
- W4220971757 cites W3038801422 @default.
- W4220971757 cites W3039098462 @default.
- W4220971757 cites W3080248008 @default.
- W4220971757 cites W3087231681 @default.
- W4220971757 cites W3092725391 @default.
- W4220971757 cites W3105938624 @default.
- W4220971757 cites W3114227877 @default.
- W4220971757 cites W3118667325 @default.
- W4220971757 cites W3137957957 @default.
- W4220971757 cites W3139441238 @default.
- W4220971757 cites W4231439639 @default.
- W4220971757 doi "https://doi.org/10.1038/s41467-022-28869-6" @default.
- W4220971757 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35273166" @default.
- W4220971757 hasPublicationYear "2022" @default.
- W4220971757 type Work @default.
- W4220971757 citedByCount "24" @default.
- W4220971757 countsByYear W42209717572022 @default.
- W4220971757 countsByYear W42209717572023 @default.
- W4220971757 crossrefType "journal-article" @default.
- W4220971757 hasAuthorship W4220971757A5010731144 @default.
- W4220971757 hasAuthorship W4220971757A5012386870 @default.
- W4220971757 hasAuthorship W4220971757A5014874162 @default.
- W4220971757 hasAuthorship W4220971757A5022785909 @default.
- W4220971757 hasAuthorship W4220971757A5031877516 @default.
- W4220971757 hasAuthorship W4220971757A5050500604 @default.
- W4220971757 hasAuthorship W4220971757A5068761476 @default.
- W4220971757 hasAuthorship W4220971757A5073206123 @default.
- W4220971757 hasAuthorship W4220971757A5076923063 @default.
- W4220971757 hasAuthorship W4220971757A5091386340 @default.
- W4220971757 hasBestOaLocation W42209717571 @default.
- W4220971757 hasConcept C138631740 @default.
- W4220971757 hasConcept C155672457 @default.
- W4220971757 hasConcept C161790260 @default.
- W4220971757 hasConcept C171250308 @default.
- W4220971757 hasConcept C178790620 @default.
- W4220971757 hasConcept C185592680 @default.
- W4220971757 hasConcept C192562407 @default.
- W4220971757 hasConcept C2778402822 @default.
- W4220971757 hasConcept C45083100 @default.
- W4220971757 hasConceptScore W4220971757C138631740 @default.
- W4220971757 hasConceptScore W4220971757C155672457 @default.
- W4220971757 hasConceptScore W4220971757C161790260 @default.
- W4220971757 hasConceptScore W4220971757C171250308 @default.
- W4220971757 hasConceptScore W4220971757C178790620 @default.
- W4220971757 hasConceptScore W4220971757C185592680 @default.
- W4220971757 hasConceptScore W4220971757C192562407 @default.
- W4220971757 hasConceptScore W4220971757C2778402822 @default.
- W4220971757 hasConceptScore W4220971757C45083100 @default.
- W4220971757 hasIssue "1" @default.
- W4220971757 hasLocation W42209717571 @default.
- W4220971757 hasLocation W42209717572 @default.
- W4220971757 hasLocation W42209717573 @default.
- W4220971757 hasLocation W42209717574 @default.