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• W4220972012 abstract "The creation of inclusion complexes with Saturn-like geometries has attracted increasing attention for supramolecular systems, but expansion of the concept to nanoscale colloidal systems remains a challenge. Here, we report a strategy to assemble toroidal polyisoprene-b-poly(2-vinylpyridine) (PI-b-P2VP) block copolymer micelles with a PI core and a P2VP corona and inorganic (e.g., silica) nanoparticles of variable shape and dimensions into Saturn-like constructs with high fidelity and yield. The precise nesting of the nanoparticles between the toroidal building units is realized by virtue of hydrogen bonding and self-adaptive expansion of the flexible toroidal units enabled by a flexible, low Tg PI core. Once the toroidal units are cross-linked, the self-adaptive feature is lost and coassembly yields instead out-of-cavity bound nanoparticles. Saturn-like assemblies can also be formed along silica nanosphere-decorated cylindrical micelles or, alternatively, at the hydroxyl-functionalized termini of cylindrical micelles to yield colloidal [3]rotaxanes." @default.
• W4220972012 created "2022-04-03" @default.
• W4220972012 creator A5058247032 @default.
• W4220972012 creator A5076582889 @default.
• W4220972012 creator A5082755637 @default.
• W4220972012 date "2022-03-24" @default.
• W4220972012 modified "2023-10-15" @default.
• W4220972012 title "“Self-Adaptive” Coassembly of Colloidal “Saturn-like” Host–Guest Complexes Enabled by Toroidal Micellar Rubber Bands" @default.
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• W4220972012 doi "https://doi.org/10.1021/jacs.2c01109" @default.
• W4220972012 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35324193" @default.
• W4220972012 hasPublicationYear "2022" @default.
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