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• W4220981572 abstract "Abstract In 1965 Duwez et al. reported having generated an amorphous, stable phase of palladium-silicon in the region 15 to 23 atomic percent, at.%, silicon. These pioneering efforts have led to the development of solid materials that are now known as Bulk Metallic Glasses, BMG. In 2019 Rodríguez et al. discovered, computationally, that bulk amorphous Pd becomes magnetic, and so does porous/amorphous Pd. Puzzled by these results, the study of several solid binary systems in the Pd-rich zone was undertaken; in particular, the study of the glassy metallic alloy a -Pd $$_{100-c}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:msub> <mml:mrow /> <mml:mrow> <mml:mn>100</mml:mn> <mml:mo>-</mml:mo> <mml:mi>c</mml:mi> </mml:mrow> </mml:msub> </mml:math> Si $$_{c}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:msub> <mml:mrow /> <mml:mi>c</mml:mi> </mml:msub> </mml:math> , for $$0 le c le 22$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mrow> <mml:mn>0</mml:mn> <mml:mo>≤</mml:mo> <mml:mi>c</mml:mi> <mml:mo>≤</mml:mo> <mml:mn>22</mml:mn> </mml:mrow> </mml:math> , ( c in at.%) to see what their topology is, what their electronic properties are and to inquire about their magnetism. In this work it is shown that this metallic glass is in fact magnetic in the region $$0 le c < 15$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mrow> <mml:mn>0</mml:mn> <mml:mo>≤</mml:mo> <mml:mi>c</mml:mi> <mml:mo><</mml:mo> <mml:mn>15</mml:mn> </mml:mrow> </mml:math> . Collaterally $$alpha$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mi>α</mml:mi> </mml:math> and $$beta$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mi>β</mml:mi> </mml:math> magnetization curves are shown where the net magnetic moment is presented. The topology and the position of the first few peaks of the pair distribution functions, which agrees well with experiment, are also discussed. The BMGs produced experimentally so far are limited in size, but despite this limitation, recent industrial efforts have developed some useful devices that may revolutionize technology." @default.
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• W4220981572 date "2022-03-17" @default.
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• W4220981572 title "Ab initio studies of magnetism and topology in solid Pd-rich $${varvec{a}}$$-PdSi alloys" @default.
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• W4220981572 doi "https://doi.org/10.1038/s41598-022-08656-5" @default.
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