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- W4221006095 abstract "A series of six tripodal push-pull fluorophores with D-(π-A3) arrangement has been designed and synthesized. The structure of these fluorophores consists of a central electron-donating triphenylamine core and peripheral electron-withdrawing diazine units (pyridazine, pyrimidine, and pyrazine moieties), which are linked by an ethynylene π-spacer. The preparation of the fluorophores involves threefold Sonogashira cross-coupling reaction starting from the key tris(4-ethynylphenyl)amine intermediate. The structure and spatial arrangement of two fluorophores were completely confirmed by X-ray analysis. Thermal and electrochemical behavior of prepared fluorophores were investigated by differential scanning calorimetry and cyclic voltammetry. Their linear optical properties were examined by UV–Vis absorption, steady-state and time resolved fluorescent spectroscopy while 2 PA analysis was used for a study of the nonlinear optical response. Experimental data were supported by DFT calculations. Based on the experimental as well as theoretical data, structure-property relationships have been thoroughly revealed." @default.
- W4221006095 created "2022-04-03" @default.
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- W4221006095 date "2022-05-01" @default.
- W4221006095 modified "2023-10-16" @default.
- W4221006095 title "Triphenylamine-based fluorophores bearing peripheral diazine regioisomers. Synthesis, characterization, photophysics and two-photon absorption" @default.
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- W4221006095 doi "https://doi.org/10.1016/j.dyepig.2022.110230" @default.
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