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• W4221047899 abstract "Herein, we describe the synthesis of 5-fluoro-dihydroindolizines via dual C-F bond cleavage in a trifluoromethyl group. The photocatalytic defluorinative coupling of pyrrole-2-acetic acids and α-trifluoromethyl alkenes cleaved the first C-F bond, providing gem-difluoroalkenes bearing an unprotected pyrrole motif. Subsequently, an intramolecular SNV reaction closed the ring by forming a C-N bond concomitantly with the cleavage of the second C-F bond. Using indole-2-acetic acids as the substrates, the reactions also allow the assembly of 6-fluoro-dihydropyrido[1,2-a]indoles." @default.
• W4221047899 created "2022-04-03" @default.
• W4221047899 creator A5025849939 @default.
• W4221047899 creator A5034855606 @default.
• W4221047899 date "2022-03-17" @default.
• W4221047899 modified "2023-09-27" @default.
• W4221047899 title "Synthesis of 5-Fluoro-dihydroindolizines from Pyrrole-2-acetic Acids and Trifluoromethyl Alkenes via Dual C–F Bond Cleavage in a CF₃ Group" @default.
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• W4221047899 doi "https://doi.org/10.1021/acs.joc.2c00077" @default.
• W4221047899 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35297252" @default.
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