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- W4223903670 abstract "Stimulated Raman scattering (SRS) is known to gain coherent amplification of molecular vibrations that allow for rapid and label-free chemical imaging in the microscopy setting. However, the tightly focused laser spot has limited the detection sensitivity, partly due to the tiny interaction volume. Here, we report the use of metal-lined hollow-core fiber (MLHCF) to improve the sensitivity of SRS in sensing dilute solutions by extending the light-matter interaction volume through the fiber waveguide. With a focusing lens (100 mm FL) and 320 μm diameter fiber, we demonstrated an optimum enhancement factor of ~20 at a fiber length of 8.3 cm. More importantly, the MLHCF exhibited a significantly suppressed cross-phase modulation (XPM) background, enabling the detection of ~0.7 mM DMSO in water. Furthermore, the relationship between fiber length and SRS signal could be well explained theoretically. The fiber-enhanced SRS (FE-SRS) method may be further optimized and bears potential in the sensitive detection of molecules in the solution and gas phases." @default.
- W4223903670 created "2022-04-19" @default.
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- W4223903670 date "2022-04-14" @default.
- W4223903670 modified "2023-10-11" @default.
- W4223903670 title "Fiber-Enhanced Stimulated Raman Scattering and Sensitive Detection of Dilute Solutions" @default.
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- W4223903670 doi "https://doi.org/10.3390/bios12040243" @default.
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