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• W4223989161 abstract "Designing a thick electrode with appropriate mass loading is a prerequisite toward practical applications for lithium ion batteries (LIBs) yet suffers severe limitations of slow electron/ion transport, unavoidable volume expansion, and the involvement of inactive additives, which lead to compromised output capacity, poor rate perforamnce, and cycling instability. Herein, self-supported thick electrode composed of vertically aligned two-dimensional (2D) heterostructures (V-MXene/V2O5) of rigid Ti3C2TX MXene and pliable vanadium pentoxide are assembled via an ice crystallization-induced strategy. The vertical channels prompt fast electron/ion transport within the entire electrode; in the meantime, the 3D MXene scaffold provides mechanical robustness during lithiation/delithiation. The optimized electrodes with 1 and 5 mg cm–2 of V-MXene/V2O5 respectively deliver 472 and 300 mAh g–1 at a current density of 0.2 A g–1, rate performance with 380 and 222 mAh g–1 retained at 5 A g–1, and reliability over 800 charge/discharge cycles." @default.
• W4223989161 created "2022-04-19" @default.
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• W4223989161 date "2022-04-15" @default.
• W4223989161 modified "2023-10-17" @default.
• W4223989161 title "Design of Vertically Aligned Two-Dimensional Heterostructures of Rigid Ti₃C₂T_X MXene and Pliable Vanadium Pentoxide for Efficient Lithium Ion Storage" @default.
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• W4223989161 doi "https://doi.org/10.1021/acsnano.1c10212" @default.
• W4223989161 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35426659" @default.
• W4223989161 hasPublicationYear "2022" @default.
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