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- W4224108889 abstract "Spiropyran-bearing telechelic poly (2-isopropyl-2-oxazoline) (SP-PiPrOx-SP) was designed as a multimodal stimuli-responsive polymer. Formed via living cationic ring-opening polymerization and ester coupling of spiropyran units, the resultant SP-PiPrOx-SP had an average molecular weight of 8.0 kDa with a narrow molecular weight distribution. SP-PiPrOx-SP exhibited a sharp hydrophilic-hydrophobic thermal transition at a specific temperature. Moreover, SP-PiPrOx-SP showed reversible photochromic changes between the colorless SP-PiPrOx-SP and purple MC-PiPrOx-MC states upon UV or visible light irradiation. The addition of DBU to MC-PiPrOx-MC resulted in the formation of a stable yellow complex that did not exhibit photochromic behavior. When CO2 was added to the yellow DBU adduct of MC-PiPrOx-MC, the solution immediately changed to purple due to the dissociation of DBU from MC-PiPrOx-MC. The addition of DBU to MC-PiPrOx-MC induced dramatic changes to the thermal transition temperature. Because SP-PiPrOx-SP simultaneously shows thermal transition, photochromic, and chemoresponsive properties, the introduction of spiropyran units has great potential for the design of functional materials." @default.
- W4224108889 created "2022-04-19" @default.
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- W4224108889 date "2022-06-01" @default.
- W4224108889 modified "2023-10-02" @default.
- W4224108889 title "Multimodal stimuli-responsive behaviors of photochromic spiropyran-bearing telechelic poly(2-isopropyl-2-oxazoline)" @default.
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- W4224108889 doi "https://doi.org/10.1016/j.mtchem.2022.100884" @default.
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