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- W4224247230 abstract "A metabolic cycle-inspired hydrogel which exhibits the biomacromolecule-fueled transient volume phase transition is reported. This hydrogel has the affinity and digestive capacity for a fuel α-poly-L-lysine by incorporating acrylic acid and trypsin. The hydrogel captured fuel and transiently shrank owing to the construction of electrostatic cross-linkages. This process was inherently connected with the digestion of these cross-linkages and the release of oligo-lysine as waste, which induced the reswelling of the hydrogel at equilibrium. The transient volume change of the hydrogel realized the fuel-stimulated transient release of a payload. This study provides a strategy for engineering materials with biomacromolecule-fueled dynamic functions under the out-of-equilibrium condition." @default.
- W4224247230 created "2022-04-26" @default.
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- W4224247230 date "2022-05-03" @default.
- W4224247230 modified "2023-10-15" @default.
- W4224247230 title "Biomacromolecule‐Fueled Transient Volume Phase Transition of a Hydrogel" @default.
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- W4224247230 doi "https://doi.org/10.1002/ange.202205125" @default.
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