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- W4224253124 abstract "Understanding how to structure a porous electrode to facilitate fluid, mass, and charge transport is key to enhancing the performance of electrochemical devices, such as fuel cells, electrolyzers, and redox flow batteries (RFBs). Using a parallel computational framework, direct numerical simulations are carried out on idealized porous electrode microstructures for RFBs. Strategies to improve an electrode design starting from a regular lattice are explored. By introducing vacancies in the ordered arrangement, it is possible to achieve higher voltage efficiency at a given current density, thanks to improved mixing of reactive species, despite reducing the total reactive surface. Careful engineering of the location of vacancies, resulting in a density gradient, outperforms disordered configurations. Our simulation framework is a new tool to explore transport phenomena in RFBs, and our findings suggest new ways to design performant electrodes." @default.
- W4224253124 created "2022-04-26" @default.
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- W4224253124 date "2022-04-01" @default.
- W4224253124 modified "2023-09-26" @default.
- W4224253124 title "Less can be more: Insights on the role of electrode microstructure in redox flow batteries from two-dimensional direct numerical simulations" @default.
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- W4224253124 doi "https://doi.org/10.1063/5.0084066" @default.
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