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• W4224277840 abstract "Polymer electrolytes have attracted great interest for next-generation lithium batteries and emerging energy applications due to their prominent advantages such as superior thermal/mechanical/electrical properties, low density, easy processability, and low cost. As a type of solid-state electrolyte, polymer electrolytes can not only effectively improve the safety characteristic of batteries, but also be easily industrialized owing to their simple production process. At present, polymer electrolytes are considered to be one of the most suitable electrolytes for the commercially available lithium battery production process, whose power batteries have been produced by the Bollore Company in France. Furthermore, polymer electrolytes generally possess superior compatibility with lithium metal anodes, which is favorable to break through the ceiling of the energy density of lithium batteries. The concept of the polymer electrolyte was started in 1973.[1] reported that alkali metal salts could be dissolved in poly(ethylene oxide) (PEO) to form conductive complexes. In 1978,[2] proposed a PEO/Li salt-based polymer electrolyte with an ionic conductivity of ≈10–4 S cm–1 at 40–60 °C for lithium batteries. Since then, polymer electrolytes have undergone rapid progress. For this special issue of Macromolecular Chemistry and Physics, we hope it is timely to highlight solid-state lithium batteries and emerging next-generation batteries, which will draw a great and wide readership from the extensive field of materials, electrochemistry and clean energy. This special issue features two reviews and 12 research articles, which paints a current picture of the state-of-the-art of polymer electrolytes. With pleasure, we note that the contributions are received from both established researchers with lifelong expertise in polymer electrolytes and emerging investigators with a wealth of ideas. In one of the reviews, available in open access, Jelena Popovic summarizes dry polymer electrolytes for solid-state batteries in terms of the relevant physico-chemical properties, ionic transport mechanism, molecular structure, and interfacial issues (2100344). Guanglei Cui and colleagues review and discuss the functional applications of polymer electrolytes in high-energy-density lithium batteries (2100410). Molecular design is very important for the development of polymer electrolytes. Hiroyoshi Kawakami and colleagues present two kinds of cross-linked polyether-based electrolytes to improve the safety of lithium-ion secondary batteries (2100317). David Mecerreyes and coworkers design a boron-based single-ion gel polymer electrolyte by photopolymerization for lithium batteries (2100407). Yoichi Tominaga and co-workers design a crosslinked poly[(ethylene carbonate)-co-(ethylene oxide)]/lithium bis(fluorosulfonyl)imide based electrolyte, which exhibits both superior mechanical strength and excellent ion-conductive properties (2100327). It is well-known that compositing and doping are both powerful strategies to improve the battery properties of polymer electrolytes. Patrik Johansson and Laura C. Loaiza dope lithium salt with single-ion conducting polymer electrolytes to enhance their ion conductivity (2100419). Yoichi Tominaga and co-workers add LiNO3 into polyether electrolytes to improve the performance of all-solid-state Li metal battery (2100396). Lianqi Zhang and colleagues present a methylcellulose/polymethyl methacrylate/Al2O3 composite polymer matrix for Ni-rich cathode/lithium metal battery (2100234). Liaoyun Zhang and colleagues design a MOF-based composite all-solid-state polymer electrolyte with significantly improved comprehensive performance for dendrite-free lithium batteries (2100325). The ion transport mechanism is also a key basic scientific issue in polymer electrolytes. Monika Schönhoff and Mark P. Rosenwinkel investigate the Li transport mechanisms in ionic liquid based ternary polymer electrolytes in their open access article (2100320), providing a good theoretical guidance to improve the ionic conductivity of polymer electrolytes. Additonally, polymer electrolytes are widely used in other energy storage devices. Xianfeng Li and colleagues prepare a cross-linked poly(arylene ether sulfone) membrane for vanadium flow battery (2100338). Masahiro Yoshizawa-Fujita and co-workers study the ion conductive behavior of oligoether/zwitterion diblock copolymers/magnesium salt-based electrolytes (2100363). Kazuhide Ueno and colleagues design liquid metal/ionic liquid composite gels as mixed electronic/ionic conductors, which can be read open access (2100319). Vito Di Noto and co-workers present inorganic/organic hybrid anion conducting membranes based on ammonium-functionalized polyethylene pyrrole-polyethylene ketone copolymer (2100409). These new polymer electrolytes have not only been successfully applied in a variety of energy storage devices, but also provided many new ideas for the design of polymer electrolytes in lithium batteries. Finally, we would like to thank all of the contributing authors of this special issue. We also would like to thank Editor-in-Chief Mara Staffilani as well as Joe Krumpfer, not only for the invitation, but also for their patience while assembling the special issue. We hope that this issue will serve as an inspiration to many readers working on materials, electrochemistry and clean energy, in order to pave the way for future research directions in the rapidly growing area of polymer electrolytes. Guanglei Cui received his Ph.D. degree from the Institute of Chemistry, Chinese Academy of Sciences (CAS). He did postdoctoral research at Max-Planck-Institute for Polymer Research and Max-Planck-Institute for Solid State Research before joining Qingdao Institute of Bioenergy and Bioprocess Technology (QIBEBT), CAS in 2009. He is currently the leader of Solid Energy System Technology Center and Deputy Director of Academic Committee of QIBEBT. His research topics include sustainable energy-storage materials, all-solid-state batteries, and novel energy devices. Yoichi Tominaga is a professor at Tokyo University of Agriculture and Technology (TUAT). He was a Ph.D. graduate from Dr. Hiroyuki Ohno's group in 2000. After graduation, he took up an academic position at Tokyo Institute of Technology in 2000, worked as an assistant professor by 2007 and was appointed lecturer and associate professor of TUAT in 2007–2018. His research topics include functional polymer-based materials and related devises for energy." @default.
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• W4224277840 title "Polymer Electrolytes toward Next‐Generation Batteries" @default.
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• W4224277840 doi "https://doi.org/10.1002/macp.202200013" @default.
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