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- W4224281346 abstract "To exploit polyoxometalate (POM)-based metal-organic complexes (MOCs) with outstanding electro- and photo-chemical performances, two new bis-amide derivative N-donor ligands featuring a 'V'-like connector, 4,4'-bis(3-pyridinecarboxamide)phenylmethane (L1) and 4,4'-bis(3-pyridinecarboxamide)phenylketone (L2), were designed and reacted with Anderson-type POMs in the presence of Co(II) ions under solvothermal conditions, which generated four MOCs: [Co2(L1)2(AlMo6H5O24)]·4H2O (1), [Co2(HL1)2(H2O)6(TeMo6O24)]·2H2O (2), [Co2(HL2)2(H2O)4[AlMo6H6O24]2]·5H2O (3), and [Co2(HL2)2(H2O)6(TeMo6O24)]·2H2O (4). All the complexes showed supramolecular structures via hydrogen bond interaction, which resulted from the 2D layers for 1, the satellite-like structural units for 2 and 4, but the 1D chains for 3. In these structures, the POMs and organic ligands exhibited different coordination modes. Both 2 and 4 showed efficient ampere sensing activities for Cr(VI) with lower limits of detection of 0.029 and 0.038 μM, respectively. Complexes 1 and 2 showed good visible-light catalytic behavior toward the reduction of Cr(VI), which offers more chances for developing electrochemical sensors and photocatalysts for Cr(VI)." @default.
- W4224281346 created "2022-04-26" @default.
- W4224281346 creator A5010776860 @default.
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- W4224281346 date "2022-01-01" @default.
- W4224281346 modified "2023-10-16" @default.
- W4224281346 title "Cobalt complexes tuned by Anderson-type polyoxometalates and bis-amide derivative ligands featuring a ‘V’-like connector for efficient ampere sensing and the visible-light catalytic reduction of Cr(<scp>vi</scp>)" @default.
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- W4224281346 doi "https://doi.org/10.1039/d1dt04341b" @default.
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